I don't think 'crush' is a really fitting word.
Zant is a thoroughly toxic personality, sociopathic at least, likely borderline personality disorder.
What is possibly likely is that he desired Midna, perhaps as little more than as a display of control, or as an idealised conquest, possibly as others have said as a legitimising aspect for a usurper. It's doubtful than anybody like Zant could actually love anyone beyond his idealised image of them.
I can't see the neck snap as being related to Midna. A personality like Zant would more likely be resentful of being abandoned by Ganondorf rather than anything he might have done to Midna.