I love the music in SS! Some of my favorites were Ballad of the Goddess, Fi's theme (any version espcially the piano one), the song of the hero, romance theme, faron woods silent realm, dragon music and that music that plays after beating the imprisoned the first time when the old lady talks to you about the gate of time (it plays a few other times too but that was the first time I think).
Gosh, I loved the music in SS. In my first playthrough, I stopped a number of times mid-game just to appreciate the area themes. I've already downloaded a bunch, too. There wasn't really any music I didn't like that I can think of, actually. But these stood out, in my opinion.
-Eldin Volcano was the first one that really struck me. I love it, definitely one of my faves.
-Lanayru Desert (past and present) is nice, pretty ambient.
-Din's Power was my favorite of the harp songs
-Bamboo Island was pleasantly odd and soothing, and really Japanese-sounding
-The Gate of Time and Follow Fi themes were really beautiful and emotional.
-Certain Boss themes
For some reason, I always like the songs in Zelda games associated with Fire/Power. (Eldin Volcano, Din's Power, and one of my top favorite songs from OoT was the Bolero of Fire) I'm more drawn to those crescendo, fast tempo ones
This place is so relaxing, its nice that they put a little comfort into this area. It sort of reminds me of Ordon and Lon Lon Ranch at the same time. I also like the epic badass boss music and scenes too but Zelda makes the best villages.